Capacity fade in solid-state batteries: interphase formation and chemomechanical processes in nickel-rich layered oxide cathodes and lithium thiophosphate solid electrolytes. Redox-active cathode interphases in solid-state batteries. All-solid-state batteries with thick electrode configurations. Inducing high ionic conductivity in the lithium superionic argyrodites Li 6+ xP 1– xGe xS 5I for all-solid-state batteries. Engineering stable interfaces for three-dimensional lithium metal anodes. Porous carbon hosts for lithium–sulfur batteries. Nanoscale nucleation and growth of electrodeposited lithium metal. Interfacial modification of Li/garnet electrolyte by a lithiophilic and breathing interlayer. Electrochemical behaviors and reaction mechanism of nanosilver with lithium. Li-alloy based anode materials for Li secondary batteries. Ultrafine silver nanoparticles for seeded lithium deposition toward stable lithium metal anode. Wrinkled graphene cages as hosts for high-capacity Li metal anodes shown by cryogenic electron microscopy. ![]() Selective deposition and stable encapsulation of lithium through heterogeneous seeded growth. ![]() Long cycle life and dendrite-free lithium morphology in anode-free lithium pouch cells enabled by a dual-salt liquid electrolyte. Accommodating lithium into 3D current collectors with a submicron skeleton towards long-life lithium metal anodes. Measuring the Coulombic efficiency of lithium metal cycling in anode-free lithium metal batteries. Anode-free rechargeable lithium metal batteries. A large deformation elastic–viscoplastic model for lithium. Elastic, plastic, and creep mechanical properties of lithium metal. ![]() Masias, A., Felten, N., Garcia-Mendez, R., Wolfenstine, J. Mechanical deformation of a lithium-metal anode due to a very stiff separator. Lithium metal anodes for rechargeable batteries. Pathways for practical high-energy long-cycling lithium metal batteries. Insights into interfacial stability of Li 6PS 5Cl solid electrolytes with buffer layers. Interfacial reactivity and interphase growth of argyrodite solid electrolytes at lithium metal electrodes. Solvent-engineered design of argyrodite Li 6PS 5X (X = Cl, Br, I) solid electrolytes with high ionic conductivity. Suppression of H 2S gas generation from the 75Li 2S♲5P 2S 5 glass electrolyte by additives. Sulfide solid electrolyte with favorable mechanical property for all-solid-state lithium battery. Interfaces between cathode and electrolyte in solid state lithium batteries: challenges and perspectives. Electrolytes and interphases in Li-ion batteries and beyond. A low ride on processing temperature for fast lithium conduction in garnet solid-state battery films. Pfenninger, R., Struzik, M., Garbayo, I., Stilp, E. High electronic conductivity as the origin of lithium dendrite formation within solid electrolytes. Negating interfacial impedance in garnet-based solid-state Li metal batteries. Sulfide solid electrolytes for lithium battery applications. High-power all-solid-state batteries using sulfide superionic conductors. Performance and cost of materials for lithium-based rechargeable automotive batteries. Schmuch, R., Wagner, R., Hörpel, G., Placke, T. A prototype pouch cell (0.6 Ah) thus prepared exhibited a high energy density (>900 Wh l −1), stable Coulombic efficiency over 99.8% and long cycle life (1,000 times). A warm isostatic pressing technique was also introduced to improve the contact between the electrode and the electrolyte. In our full-cell demonstrations, we employed a high-Ni layered oxide cathode with a high specific capacity (>210 mAh g −1) and high areal capacity (>6.8 mAh cm −2) and an argyrodite-type sulfide electrolyte. We show that the thin Ag–C layer can effectively regulate Li deposition, which leads to a genuinely long electrochemical cyclability. Here we report that a high-performance all-solid-state lithium metal battery with a sulfide electrolyte is enabled by a Ag–C composite anode with no excess Li. However, undesirable Li dendrite growth and low Coulombic efficiency impede their practical application. ![]() An all-solid-state battery with a lithium metal anode is a strong candidate for surpassing conventional lithium-ion battery capabilities.
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